How can I load (copy) the data that is present in the GridView into the DataTable? I am trying to do this as I am unable to delete a unbounded row in the GridView. I am planning on loading the
DataTable from GridView and delete a row from the datatable and load the newly formed data with the GridView

 Any alternative solutions to this is greatly appreciated

Thanks :)

Try the GridView.DataSource and cast it to a DataTable.