You need to look at the drive that the Primary file group is on... physically, it is full. You either need to remove something from it or make a secondary file group on another drive. You may be able to recover some space if your log is on the same drive by doing a backup to decrease the space used and then shrink the log. Then, perhaps, move the log to another drive which will also have the benefit of increasing performance on the server overall.
--Jeff Moden
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